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Stamenkovic, B., Meng, Y. S., Moreau, P. & Gaubicher, J. (2024) Communication-Fueling from the Electrochemistry of Halide Solid Electrolytes. J. Electrochem. Soc. 171 050554. 
Added by: Richard Baschera (2024-06-10 10:03:53)   Last edited by: Richard Baschera (2024-06-10 10:06:09)
Type de référence: Article
DOI: 10.1149/1945-7111/ad4c99
Numéro d'identification (ISBN etc.): 0013-4651, 1945-7111
Clé BibTeX: Stamenkovic2024
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Mots-clés: all solid state battery, halide electrolyte, LiFePO4 silicium anode less, redox electrolyte, sacrificial
Créateurs: Gaubicher, Meng, Moreau, Stamenkovic
Collection: J. Electrochem. Soc.
Consultations : 5/5
Indice de consultation : 21%
Indice de popularité : 5.25%
Liens URLs     https://www.webofs ... OS:001233776500001
Unveiling the electrochemistry of solid-state Li2ZrCl6 halide electrolyte, we reveal its triple function as an ion conductor and a supplementary reversible, and sacrificial, electron source/sink. This groundbreaking discovery leads to a remarkable long-term enhancement of the specific capacity of industry-relevant heavily loaded LiFePO4 electrodes by several tens of percent, while significantly amplifying that of Si-based or anode-less full cells through effective compensation for side reactions. We show that these effects can potentially be tuned by adjusting the initial xLiCl-ZrCl4 composition of the solid electrolyte, which may thus become a new and mighty parameter for balancing the two electrodes. (c) 2024 The Author(s). Published on behalf of The Electrochemical Society by IOP Publishing Limited. This is an open access article distributed under the terms of the Creative Commons Attribution 4.0 License (CC BY,, which permits unrestricted reuse of the work in any medium, provided the original work is properly cited.
Num Pages: 4 Place: Pennington Publisher: Electrochemical Soc Inc Web of Science ID: WOS:001233776500001
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